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Author Mercer, Ian P.
Source United States Department of Energy Office of Scientific and Technical Information
Content type Text
Language English
Subject Keyword CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSICS ♦ ATOMIC AND MOLECULAR PHYSICS ♦ COHERENT RADIATION ♦ ENERGY TRANSFER ♦ MAPPING ♦ MATHEMATICAL SOLUTIONS ♦ MIXING ♦ MOLECULAR STRUCTURE ♦ QUANTUM STATES ♦ SENSITIVITY ♦ VISIBLE RADIATION ♦ ELECTROMAGNETIC RADIATION ♦ RADIATIONS
Abstract A generalized approach is derived for the analysis of angle-resolved coherent optical wave mixing. Remarkably with this, a signal is calculated to remain efficiently generated for the arbitrary evolution of a quantum superposition state and for energy transfer spanning an ultrawide bandwidth in solution. This approach is compact and applies across matter processes and wave-mixing schemes. A high sensitivity and sampling rate are shown to be intrinsic to angle-resolved wave mixing and an angle-resolved six-wave mixing scheme is proposed for the mapping of molecular structure.
ISSN 10502947
Educational Use Research
Learning Resource Type Article
Publisher Date 2010-10-15
Publisher Place United States
Journal Physical Review. A
Volume Number 82
Issue Number 4


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